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Abstract The magnetic ground state of the pyrochlore Yb 2 GaSbO 7 has not been established. The persistent spin fluctuations observed by muon spin-relaxation measurements at low temperatures have not been adequately explained for this material using existing theories for quantum magnetism. Here we report on the synthesis and characterisation of Yb 2 GaSbO 7 to revisit the nature of the magnetic ground state. Through DC and AC magnetic susceptibility, heat capacity, and neutron scattering experiments, we observe evidence for a dynamical ground state that makes Yb 2 GaSbO 7 a promising candidate for disorder-induced spin-liquid or spin-singlet behaviour. This state is quite fragile, being tuned to a splayed ferromagnet in a modest magnetic field μ 0 H c ~ 1.5 T.more » « less
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Bai, X. ; Paddison, J. A. M. ; Kapit, E. ; Koohpayeh, S. M. ; Wen, J. -J. ; Dutton, S. E. ; Savici, A. T. ; Kolesnikov, A. I. ; Granroth, G. E. ; Broholm, C. L. ; et al ( , Physical Review Letters)
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Ge, L. ; Flynn, J. ; Paddison, J. A. ; Stone, M. B. ; Calder, S. ; Subramanian, M. A. ; Ramirez, A. P. ; Mourigal, M. ( , Physical Review B)
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Hallas, A. M. ; Paddison, J. A. ; Silverstein, H. J. ; Goodwin, A. L. ; Stewart, J. R. ; Wildes, A. R. ; Cheng, J. G. ; Zhou, J. S. ; Goodenough, J. B. ; Choi, E. S. ; et al ( , Physical Review B)